论文标题
揭示粘性和多稳定性滞后在粘合剂,名义平坦的冲击中的共同作用:一项组合数值和实验性研究
Revealing the co-action of viscous and multistability hysteresis in an adhesive, nominally flat punch: A combined numerical and experimental study
论文作者
论文摘要
众所周知,粘弹性会引起裂纹闭合的明显滞后,当弹性体与平坦,刚性,粘合剂的反面接触时,打开。粘合性滞后的单独起源是小规模的弹性多稳定性。在这里,我们研究了一种同时起作用的系统。具体而言,我们比较了界面力的模拟和实验测量的时间演化,以及软弹性体和刚性平坦的冲击之间的真实接触区域,并将其添加了小规模的单鞋体粗糙度。为此,我们进一步促进了绿色的函数分子动力学方法,并扩展了最近开发的成像技术,以阐明拉力过程的速率和预努力依赖性。我们的结果表明,当地形接触的马鞍点接触时,滞后会大大增强,但是,粘弹性会阻碍粘弹性,并且可能需要足够大的预加载。预计在宏观聚合物接触中会发生类似的粘性和多稳定性效应,例如,对于压力敏感的粘合剂和现代的粘合剂夹杂装置。
Viscoelasticity is well known to cause significant hysteresis of crack closure and opening when an elastomer is brought in and out of contact with a flat, rigid, adhesive counterface. A separate origin of adhesive hysteresis is small-scale, elastic multistability. Here, we study a system in which both mechanisms act concurrently. Specifically, we compare the simulated and experimentally measured time evolution of the interfacial force and the real contact area between a soft elastomer and a rigid, flat punch, to which small-scale, single-sinusoidal roughness is added. To this end, we further the Green's function molecular dynamics method and extend recently developed imaging techniques to elucidate the rate- and preload-dependence of the pull-off process. Our results reveal that hysteresis is much enhanced when the saddle points of the topography come into contact, which, however, is impeded by viscoelastic forces and may require sufficiently large preloads. A similar coaction of viscous- and multistability effects is expected to occur in macroscopic polymer contacts and to be relevant, e.g., for pressure-sensitive adhesives and modern adhesive gripping devices.