论文标题
超导和电荷密度波之间的动态相互作用:一项相干驱动的2H-NBSE2和LA2-XSRXCUO4的非线性Terahertz研究
Dynamical interplay between superconductivity and charge-density-wave: a nonlinear terahertz study of coherently-driven 2H-NbSe2 and La2-xSrxCuO4
论文作者
论文摘要
2H-NBSE2是一种原型系统,其中超导性和电荷密度波(CDW)共存并互相竞争。特别是,这种相互作用也体现在它们的动态波动中。结果,将超导幅度波动(即希格斯模式)推在准片段连续体下方,从而使其成为可以通过拉曼散射观察到的连贯的激发。在本研究中,我们一致地驱动了这两个顺序的集体振荡,并在时域中在驱动状态中可视化它们的相互作用。我们发现,这两种集体模式均导致Terahertz第三次谐波生成(THG)和THG信号在TC以下干扰,从而导致综合THG信号的抗谐振。动态的金兹堡 - 兰道模型表明,在抗呼声周围驱动的希格斯振荡与驱动的CDW振荡之间的周期性能量转移是可能的。除2H-NBSE2外,我们还研究了一个不足的LA2-XSRXCUO4(X〜0.12),超出了THG的扰动状态。 TC下方观察到两个THG来源之间的类似干扰。尽管在这些实验中可能还有其他THG来源,但我们的结果说明了耦合模式在Terahertz Thg过程中的作用,以及通过此类耦合进行连贯控制的诱人可能性。
2H-NbSe2 is an archetypal system in which superconductivity and charge-density-wave (CDW) coexist and compete macroscopically with each other. In particular, this interplay also manifests in their dynamical fluctuations. As a result, the superconducting amplitude fluctuations (i.e. Higgs mode) is pushed below the quasiparticle continuum, allowing it to become a coherent excitation observable by Raman scattering. In the present study, we coherently drive the collective oscillations of the two orders and visualize their interplay in the driven states in the time domain. We find that both collective modes contribute to terahertz third harmonic generation (THG) and the THG signals interfere below Tc, leading to an anti-resonance of the integrated THG signal. The dynamical Ginzburg-Landau model suggests that around the anti-resonance a periodic energy transfer between the driven Higgs oscillations and the driven CDW oscillations is possible. In addition to 2H-NbSe2, we also studied an underdoped La2-xSrxCuO4 (x ~ 0.12) driven beyond the perturbative regime of THG. A similar interference between two sources of THG is observed below Tc. While there might be additional sources of THG in these experiments, our results illustrate the roles of coupled modes in the terahertz THG process and the tantalizing possibility of coherent control via such couplings.