论文标题

钻石中的电信O波段发射器

A telecom O-band emitter in diamond

论文作者

Mukherjee, Sounak, Zhang, Zi-Huai, Oblinsky, Daniel G., de Vries, Mitchell O., Johnson, Brett C., Gibson, Brant C., Mayes, Edwin L. H., Edmonds, Andrew M., Palmer, Nicola, Markham, Matthew L., Gali, Ádám, Thiering, Gergő, Dalis, Adam, Dumm, Timothy, Scholes, Gregory D., Stacey, Alastair, Reineck, Philipp, de Leon, Nathalie P.

论文摘要

钻石的彩色中心是量子技术的有前途的平台。到目前为止,大多数钻石中的彩色中心都在可见的或近红​​外的波长范围内发现,这与长距离纤维通信不兼容,并且不利于生物组织中的成像。在这里,我们报告了对电信O波段中排放的新颜色中心的实验性观察,我们在硅掺杂的散装单晶钻石和微钻石中观察到。结合吸收和光致发光测量值,我们在1221 nm处确定了零子线和由42 MeV隔开的声子复制品。使用瞬态吸收光谱法,我们测量激发态寿命约为270 ps,并观察到长寿命的基线,这可能是从间间穿越到另一个自旋歧管的长期基线。

Color centers in diamond are promising platforms for quantum technologies. Most color centers in diamond discovered thus far emit in the visible or near-infrared wavelength range, which are incompatible with long-distance fiber communication and unfavorable for imaging in biological tissues. Here, we report the experimental observation of a new color center that emits in the telecom O-band, which we observe in silicon-doped bulk single crystal diamonds and microdiamonds. Combining absorption and photoluminescence measurements, we identify a zero-phonon line at 1221 nm and phonon replicas separated by 42 meV. Using transient absorption spectroscopy, we measure an excited state lifetime of around 270 ps and observe a long-lived baseline that may arise from intersystem crossing to another spin manifold.

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