论文标题

危险氧化锌:ENZ区域中的非线性反射和透射测量和建模

Gallium-doped Zinc Oxide: Nonlinear Reflection and Transmission Measurements and Modeling in the ENZ Region

论文作者

Ball, Adam, Secondo, Ray, Diroll, Benjamin T., Fomra, Dhruv, Ding, Kai, Avrutin, Vitaly, Ozgur, Umit, Kinsey, Nathaniel

论文摘要

数十年来,已寻求强大的非线性材料,以应用电信,传感和量子光学材料。凝胶氧化锌是一种II-VI透明导电氧化物,显示出有希望的非线性,类似于氧化二锡锡和铝掺杂的氧化锌,用于电信带。在这里,我们探索其在零(ENZ)附近的Epsilon中的非线性,并显示N2,在200-300 nm薄膜上,IR泵送IR泵送的eff值在4.5x10-3 cm2gw-1上。用白光源探针在近IR中测量非线性变化和反射,而近IIR中令人兴奋的是时间和波长的数据。厚度,光损失和ENZ交叉波长的三个膜是数值建模的,并将其与实验数据进行了比较,显示了分散和时间松弛的一致性。此外,我们讨论了厚膜的ENZ周围发生的最佳激发和探测波长,但对于薄膜,我们的模型提供了额外的探索自由度。获得准确的非线性测量是一项困难且耗时的任务,我们的方法在本文中为社区提供了实验性和建模的数据,以获得感兴趣的ENZ材料。

Strong nonlinear materials have been sought after for decades for applications in telecommunications, sensing, and quantum optics. Gallium-doped zinc oxide is a II-VI transparent conducting oxide that shows promising nonlinearities similar to indium tin oxide and aluminum-doped zinc oxide for the telecommunications band. Here we explore its nonlinearities in the epsilon near zero (ENZ) region and show n2,eff values on the order of 4.5x10-3 cm2GW-1 for IR pumping on 200-300 nm thin films. Measuring nonlinear changes in transmission and reflection with a white light source probe in the near-IR while exciting in the near-IR provides data in both time and wavelength. Three films varying in thickness, optical loss, and ENZ crossover wavelength are numerically modeled and compared to experimental data showing agreement for both dispersion and temporal relaxation. In addition, we discuss optimal excitation and probing wavelengths occur around ENZ for thick films but are red-shifted for thin films where our model provides an additional degree of freedom to explore. Obtaining accurate nonlinear measurements is a difficult and time-consuming task where our method in this paper provides experimental and modeled data to the community for an ENZ material of interest.

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