论文标题

两个不同的电荷密度波顺序和加压中的新出现的超导性可爱

Two Distinct Charge Density Wave Orders and Emergent Superconductivity in Pressurized CuTe

论文作者

Wang, Shuyang, Wang, Qing, An, Chao, Zhou, Yonghui, Zhou, Ying, Chen, Xuliang, Hao, Ning, Yang, Zhaorong

论文摘要

在超导粉末和Kagome CSV3SB5中发现了多个电荷密度波(CDW)订单,为研究CDW和超导性的相互作用提供了独特的环境,并改变了我们对其性质的看法。在这里,我们报告了一项高压研究,该研究通过超温度(400 mk)电运输和温度依赖性的拉曼光谱测量和第一原则计算,对准二维CDW材料可爱。我们提供了可靠的证据,表明原始的CDW顺序(CDW1)在〜6.5 GPA时转化为独特的CDW阶(CDW2)。计算表明,CDW1的驱动力是由于嵌套效应引起的,CDW2的驱动力可能是由于电子相关相互作用引起的。引人注目的是,使用圆顶样相图观察到压力诱导的超导性,其过渡将显示出从CDW1到CDW2的交叉范围的非凡拓宽。这些结果表明,加压可爱为理解多个CDW和超导性的复杂相互作用提供了一个有希望的操场。

The discovery of multiple charge-density-wave (CDW) orders in superconducting cuprates and Kagome CsV3Sb5 has offered a unique milieu for studying the interplay of CDW and superconductivity and altered our perspective on their nature. Here, we report a high-pressure study of quasi-one-dimensional CDW material CuTe through ultralow-temperature (400 mK) electrical transport and temperature-dependent Raman spectroscopy measurements and first-principles calculations. We provide solid evidence that the pristine CDW order (CDW1) transforms into a distinct CDW order (CDW2) at ~6.5 GPa. Calculations show that the driving force of CDW1 is due to the nesting effect and that of CDW2 probably arises from the electronic correlated interaction. Strikingly, pressure-induced superconductivity is observed with a dome-like phase diagram and its transition displays an extraordinary broadening along with the crossover from CDW1 to CDW2. These results demonstrate that pressurized CuTe provides a promising playground for understanding the intricated interplay of multiple CDWs and superconductivity.

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