论文标题

在非线性光子系统中,用于第三次谐波生成的多模非框架,包括2D材料

Multimode non-Hermitian framework for third harmonic generation in nonlinear photonic systems comprising 2D materials

论文作者

Christopoulos, Thomas, Kriezis, Emmanouil E., Tsilipakos, Odysseas

论文摘要

现代纳米光子学中的谐振结构是非热(泄漏和有损),并支持准模式。此外,当代空腔经常包括2D材料,以利用并共同增强其非线性特性或提供可调性。由于其无限薄的性质和强烈的分散,此类材料增加了进一步的建模复杂性。在这里,提出了一种有效分析纳米颗粒和纳米式元素中的第三次谐波产生(THG)的形式主义。它基于数值计算纳米结构中的准模式,它是通用的,并且与文献中传统的耦合模式理论方法相反,它对转换过程中涉及的共振数量没有任何先前的假设。该框架的功能通过两个选定的示例显示:一个单个散点器和一个定期的跨表面,用于其高三阶非线性。在这两种情况下,都获得了与全波非线性模拟的良好一致性。所提出的框架可能构成一个宝贵的工具,可以在纳米光结构中获得对频率产生过程的物理见解,并为实现巨大提高的THG效率提供指南。

Resonant structures in modern nanophotonics are non-Hermitian (leaky and lossy), and support quasinormal modes. Moreover, contemporary cavities frequently include 2D materials to exploit and resonantly enhance their nonlinear properties or provide tunability. Such materials add further modeling complexity due to their infinitesimally thin nature and strong dispersion. Here, a formalism for efficiently analyzing third harmonic generation (THG) in nanoparticles and metasurfaces incorporating 2D materials is proposed. It is based on numerically calculating the quasinormal modes in the nanostructure, it is general, and does not make any prior assumptions regarding the number of resonances involved in the conversion process, in contrast to conventional coupled-mode theory approaches in the literature. The capabilities of the framework are showcased via two selected examples: a single scatterer and a periodic metasurface incorporating graphene for its high third-order nonlinearity. In both cases, excellent agreement with full-wave nonlinear simulations is obtained. The proposed framework may constitute an invaluable tool for gaining physical insight into the frequency generation process in nano-optic structures and providing guidelines for achieving drastically enhanced THG efficiency.

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