论文标题

微重力的水泡,测量气泡尺寸

Aqueous foams in microgravity, measuring bubble sizes

论文作者

Pasquet, Marina, Galvani, Nicolo, Pitois, Olivier, Cohen-Addad, Sylvie, Höhler, Reinhard, Chieco, Anthony T., Dillavou, Sam, Hanlan, Jesse M., Durian, Douglas J., Rio, Emmanuelle, Salonen, Anniina, Langevin, Dominique

论文摘要

该论文描述了一项微重力泡沫的研究,其气泡尺寸分布由于扩散气体交换而演变。我们关注从泡沫表面图像确定的气泡的大小与散装泡沫中气泡大小确定的气泡之间的比较,这些气泡的大小是根据弥漫性传播光谱(DTS)确定的。从泡沫表面的图像中提取气泡尺寸分布非常困难,因此我们使用了三种不同的过程:手动分析,使用定制的Python脚本和机器学习分析的自动分析。一旦确定了各种陷阱并考虑到所有三个程序,所有三个程序都会在误差栏内产生相同的结果。 DTS仅允许确定平均气泡半径,该气泡半径与光子传输均值免费路径$ \ ell^*$成正比。先前针对无限横向范围的平板样品得出的测得的漫射传输光强度与{$ \ ell^*$}之间的关系不适用于微重力实验中使用的细胞的立方几何形状。已经得出并应用了具有特定光学边界条件的弥漫强度的新的更通用的表达,以确定平均气泡半径。从DTS推导出的平均气泡半径和在样品表面测得的气泡相同的平均半径的时间演变在整个浓缩过程中都非常一致。最后,进行了地面实验,以比较散装湿泡沫中的气泡尺寸分布,并在其表面上很短,以至于扩散气体交换微不足道。发现它们是相似的,证实在表面看到的气泡代表了散装泡沫气泡。

The paper describes a study of wet foams in microgravity whose bubble size distribution evolves due to diffusive gas exchange. We focus on the comparison between the size of bubbles determined from images of the foam surface and the size of bubbles in the bulk foam, determined from Diffuse Transmission Spectroscopy (DTS). Extracting the bubble size distribution from images of a foam surface is difficult so we have used three different procedures : manual analysis, automatic analysis with a customized Python script and machine learning analysis. Once various pitfalls were identified and taken into account, all the three procedures yield identical results within error bars. DTS only allows the determination of an average bubble radius which is proportional to the photon transport mean free path $\ell^*$. The relation between the measured diffuse transmitted light intensity and {$\ell^*$} previously derived for slab-shaped samples of infinite lateral extent does not apply to the cuboid geometry of the cells used in the microgravity experiment. A new more general expression of the diffuse intensity transmitted with specific optical boundary conditions has been derived and applied to determine the average bubble radius. The temporal evolution of the average bubble radii deduced from DTS and of the same average radii of the bubbles measured at the sample surface are in very good agreement throughout the coarsening. Finally, ground experiments were performed to compare bubble size distributions in a bulk wet foam and at its surface at times so short that diffusive gas exchange is insignificant. They were found to be similar, confirming that bubbles seen at the surface are representative of the bulk foam bubbles.

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