论文标题

超薄宽带元信表面超级射击器来自范德华半米

Ultrathin Broadband Metasurface Superabsorbers from a van der Waals Semimetal

论文作者

Alfieri, Adam D., Motala, Michael J., Snure, Michael, Lynch, Jason, Kumar, Pawan, Zhang, Huiqin, Post, Susanna, Muratore, Christopher, Hendrickson, Joshua R., Glavin, Nicholas R., Jariwala, Deep

论文摘要

在可见的和近红外(NIR)中运行的超材料和元面孔为下一代光电探测器和设备提供了有前途的途径,以进行太阳能收集。尽管已经证明了使用金属和半导体的大量超材料和跨境,但在Vis-Nir范围内基于半法的跨额定面积却显然缺少。在这里,我们在实验上展示了基于大面积的宽带超浮游生物,即半金属,范德华PTSE2薄膜与电磁模拟一致。我们的结果表明,PTSE2是一种超薄且可扩展的半学,在整个Vis-NIR范围内同时拥有高指数和高灭绝。因此,在400-900 nm范围内,由介电间隔者分离的反射器上的薄膜PTSE2可吸收> 85%,而优化的2D元面则可以吸收〜97%,这是最强和最薄的宽带完美吸收剂之一。我们的结果提出了一种可伸缩的光电检测和太阳能收集的方法,证明了高指数的高指数,高灭绝的纳米级光学的效用。

Metamaterials and metasurfaces operating in the visible and near-infrared (NIR) offer a promising route towards next-generation photodetectors and devices for solar energy harvesting. While numerous metamaterials and metasurfaces using metals and semiconductors have been demonstrated, semimetals-based metasurfaces in the vis-NIR range are notably missing. Here, we experimentally demonstrate a broadband metasurface superabsorber based on large area, semimetallic, van der Waals PtSe2 thin films in agreement with electromagnetic simulations. Our results show that PtSe2 is an ultrathin and scalable semimetal that concurrently possesses high index and high extinction across the vis-NIR range. Consequently, the thin-film PtSe2 on a reflector separated by a dielectric spacer can absorb > 85 % for the unpatterned case and ~97 % for the optimized 2D metasurface in the 400-900 nm range making it one of the strongest and thinnest broadband perfect absorbers to date. Our results present a scalable approach to photodetection and solar energy harvesting, demonstrating the practical utility of high index, high extinction semimetals for nanoscale optics.

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