论文标题
通过量子干涉测量学目睹纠缠的两光子吸收
Witnessing Entangled Two-Photon Absorption via Quantum Interferometry
论文作者
论文摘要
最近的研究表明,在实验性的两光子吸收光谱中,使用非古典光状态(例如纠缠的光子对)可能会开放新的令人兴奋的途径。尽管对纠缠的两光子吸收(ETPA)进行了几项实验研究,但关于是否真正观察到ETPA仍然存在激烈的争论。这场有趣的辩论已经引起,主要是因为最近有人争辩说,诸如散射或热频段吸收之类的单光子损失机制可能模仿了预期的纠缠 - 光子线性吸收行为。在这项工作中,我们专注于ETPA的传输测量,并在评估ETPA的背景下探索三个不同的两光子量子干涉仪。我们证明所谓的N00N状态配置是对线性(单光子)损失不敏感的唯一一种。值得注意的是,我们的结果表明,N00N状态可能成为量子光谱的潜在强大工具,并将其作为在任意样本中ETPA认证的有力候选者。
Recent investigations suggest that the use of non-classical states of light, such as entangled photon pairs, may open new and exciting avenues in experimental two-photon absorption spectroscopy. Despite several experimental studies of entangled two-photon absorption (eTPA), there is still a heated debate on whether eTPA has truly been observed. This interesting debate has arisen, mainly because it has been recently argued that single-photon-loss mechanisms, such as scattering or hot-band absorption may mimic the expected entangled-photon linear absorption behavior. In this work, we focus on transmission measurements of eTPA, and explore three different two-photon quantum interferometers in the context of assessing eTPA. We demonstrate that the so-called N00N-state configuration is the only one amongst those considered insensitive to linear (single-photon) losses. Remarkably, our results show that N00N states may become a potentially powerful tool for quantum spectroscopy, and place them as a strong candidate for the certification of eTPA in an arbitrary sample.