论文标题

非绝热波包动力学中具有几何影响的超快旋转型

Ultrafast spintronics with geometric effects in non-adiabatic wave-packet dynamics

论文作者

Tu, Matisse Wei-Yuan, Lin, Li-Sheng, Wang, Chung-Yu, Chou, Jyh-Pin, Wei, Sin-Yi, Tu, Chien-Ming, Kuo, Chia-Nung, Lue, Chin-Shan, Luo, Chih-Wei

论文摘要

我们通过激光脉冲在量子材料中带来的量子材料的几何特性来指导超铁的非绝热过程的动物动物,我们扩展了一个波动包装的传输理论,以前在绝热政权中良好地建立了良好的型号,该理论是在实质性地捕获的,该理论是在实质性地捕获的频带的几何特性,以使其具有交易型和非放射状态。这种扩展促进了我们研究表现出显微镜谱系效应的宏观方式,这些方式突出了非绝热驱动器的特殊能力。这些包括关闭激光脉冲后,包括到当前速率的刻痕​​数量以及诱导固有的宏观自旋极化,并且无法通过绝热过程无法达到方向。特别是,微观的几何固有自旋相干性显示出宏观光电的自旋介导的部分的基础。通过与Rashba自旋轨道耦合的示例的明确计算,在光电流的各向异性方面,旋转介导的部分与非旋转介导的部分可辨别。据称在RashBA示例之外适用的上述理论结果背后的工作原理被蒸馏以检查为SNSE收集的实验数据,表现出相当大的各向异性效应。观察到理论与实验之间的一致性,铺平了进一步探索上述方向的方式。

Motivated by the intriguing possibilities of steering ultrafast non-adiabatic processes through the geometric properties of bands in quantum materials by laser pulses, we extend a wave-packet transport theory, previously well-established in the adiabatic regime that intuitively captured geometric properties of bands, to the transient and non-adiabatic regime. This extension facilitates us to investigate macroscopic ways of manifesting microscopic band-geometric effects that highlight the special capability of non-adiabatic drivings not available to adiabatic drivings. These include imprinting band-geometric properties to the current rate after switching off the laser pulses and the induction of intrinsic macroscopic spin polarisation with an orientation not accessible by adiabatic processes. In particular, the microscopic geometrically-rooted intrinsic spin coherence is shown to underlie the spin-mediated parts of the macroscopic photocurrents. Through explicit calculations of an example with Rashba spin-orbit coupling, the spin-mediated part is shown to be discernible from the non-spin-mediated part in terms of the anisotropy of the photocurrents. Working principles behind the above theoretical results allegedly applicable beyond the Rashba example are distilled to inspect experimental data collected for SnSe, exhibiting considerable anisotropic effects. Consistency between theory and experiment is observed, paving the way of further exploration into the above intended direction.

扫码加入交流群

加入微信交流群

微信交流群二维码

扫码加入学术交流群,获取更多资源