论文标题
强相关材料的亚周期多维光谱
Sub-cycle multidimensional spectroscopy of strongly correlated materials
论文作者
论文摘要
密切相关的固体是极其复杂且引人入胜的量子系统,新状态继续出现,尤其是当与光触发器之间的相互作用相互作用时。在此相互作用中,作为超快操纵物质在PHZ量表上操纵物质的工具,子激光周期电子响应特别有吸引力。在这里,我们介绍了一种新型的非线性多维光谱,这使我们能够揭示与较少循环红外脉冲相互作用的紧密相关系统的亚周期动力学,以及在亚前前时间尺度上演变的不同相关状态之间的复杂相互作用。我们证明,单个粒子亚周期电子响应对相关的多体动力学非常敏感,并可以直接访问许多身体响应功能。对于在超短,激烈的电场瞬变的影响下的二维Hubbard模型,我们证明我们的方法可以在亚周期时间尺度上解决局部化和离域多体状态之间的电荷和能量流程,并遵循激光脉冲结束后高度相关状态生存的途径。我们的发现为成像制度和操纵强烈相关的材料以光速率而开辟了道路,除了浮雕工程中采用的多循环方法之外,亚周期响应是访问许多人体现象的关键工具。
Strongly correlated solids are extremely complex and fascinating quantum systems, where new states continue to emerge, especially when interaction with light triggers interplay between them. In this interplay, sub-laser-cycle electron response is particularly attractive as a tool for ultrafast manipulation of matter at PHz scale. Here we introduce a new type of non-linear multidimensional spectroscopy, which allows us to unravel the sub-cycle dynamics of strongly correlated systems interacting with few-cycle infrared pulses and the complex interplay between different correlated states evolving on the sub-femtosecond time-scale. We demonstrate that single particle sub-cycle electronic response is extremely sensitive to correlated many-body dynamics and provides direct access to many body response functions. For the two-dimensional Hubbard model under the influence of ultra-short, intense electric field transients, we demonstrate that our approach can resolve pathways of charge and energy flow between localized and delocalized many-body states on the sub-cycle time scale and follow the creation of a highly correlated state surviving after the end of the laser pulse. Our findings open a way towards a regime of imaging and manipulating strongly correlated materials at optical rates, beyond the multi-cycle approach employed in Floquet engineering, with the sub-cycle response being a key tool for accessing many body phenomena.