论文标题
S = 1/2的QUASIKAGOME晶格CERH1-XPDXSN中的量子临界旋转液样行为,使用MUON自旋松弛和中子散射研究
Quantum critical spin-liquid-like behavior in S = 1/2 quasikagome lattice CeRh1-xPdxSn investigated using muon spin relaxation and neutron scattering
论文作者
论文摘要
我们介绍了Muon Spin放松($μ$ SR)和基于CE的Quasikagome晶格CERH $ _ {1-x} $ pd $ _ {x} $ sn($ x = 0.1 $ to 0.75)上的MUON SPIN放松($μ$ SR)和中子散射的结果。我们的ZF- $μ$ SR结果显示,静态远程磁性顺序的缺乏降至0.05〜K,$ x = 0.1 $单晶。动态自旋波动的弱温度依赖性平台低于0.2〜 k,ZF- $μ$ SR及其纵向场(LF)依赖性在0和3〜 kg之间的依赖性,即使在$ = 0.05〜k的情况下,动态自旋波动也持续存在,即使没有静态磁性顺序。另一方面,$ c _ {\ text {4f}} $/$ t $在0.9〜k以下冷却时以-log $ t $的增加,在0.13〜K下通过广泛的最大值,并在进一步冷却时略微降低。 AC敏感性还表现出0.16〜K处的频率独立宽峰值,这在$ C $方向上是在应用的场上$ h $的突出峰。因此,我们认为,$ x = 0.1 $的这种行为(即,旋转放松率($λ$)低于0.2〜k的高原($λ$)和$ c _ {\ text {4f}} $ 0.13〜k以下的线性$ t $依赖性可以归因于金属旋转式(sl)的基础,这是一个沮丧的点状态。 LF- $ $ $ SR的研究表明,kagome平面旋转波动是造成SL行为的原因。 $ x $ = 0.1的低能量非弹性中子散射(INS)揭示了无间隙的磁激发,这也由$ c _ {\ text {4f}} $与$ t^{1.1} $成比例的行为所支持。
We present the results of muon spin relaxation ($μ$SR) and neutron scattering on the Ce-based quasikagome lattice CeRh$_{1-x}$Pd$_{x}$Sn ($x=0.1$ to 0.75). Our ZF-$μ$SR results reveal the absence of static long-range magnetic order down to 0.05~K in $x = 0.1$ single crystals. The weak temperature-dependent plateaus of the dynamic spin fluctuations below 0.2~K in ZF-$μ$SR together with its longitudinal-field (LF) dependence between 0 and 3~kG indicate the presence of dynamic spin fluctuations persisting even at $T$ = 0.05~K without static magnetic order. On the other hand, $C_{\text{4f}}$/$T$ increases as --log $T$ on cooling below 0.9~K, passes through a broad maximum at 0.13~K and slightly decreases on further cooling. The ac-susceptibility also exhibits a frequency independent broad peak at 0.16~K, which is prominent with an applied field $H$ along $c$-direction. We, therefore, argue that such a behavior for $x=0.1$ (namely, a plateau in spin relaxation rate ($λ$) below 0.2~K and a linear $T$ dependence in $C_{\text{4f}}$ below 0.13~K) can be attributed to a metallic spin-liquid (SL) ground state near the quantum critical point in the frustrated Kondo lattice. The LF-$μ$SR study suggests that the out of kagome plane spin fluctuations are responsible for the SL behavior. Low energy inelastic neutron scattering (INS) of $x$ = 0.1 reveals gapless magnetic excitations, which are also supported by the behavior of $C_{\text{4f}}$ proportional to $T^{1.1}$ down to 0.06~K.