论文标题
在空间不均匀培养基中的等离子的半古老理论
Semiclassical theory for plasmons in spatially inhomogeneous media
论文作者
论文摘要
实验技术的最新进展使血浆中的量子状态可访问。由于等离子对应于集体电子激发,因此电子电子相互作用在其理论描述中起着至关重要的作用。在随机阶段近似中,这种相互作用是通过运动方程组并入的,该方程式必须自一求解。对于均质培养基,可以使用傅立叶变换发现分析解决方案,从而引起Lindhard理论。当介质在空间上不均匀时,这是不再可能的,并且经常使用数值方法,但是这些方法仅限于较小的系统。在本文中,我们提出了一种基于半经典(或WKB)近似值的不均匀介质中散装等离子体的新型半分析方法,当电荷密度平稳变化时,该方法适用。通过自愿求解运动方程,我们可以通过空间变化的费米波向量获得Lindhard理论的表达。该派生涉及从操作员传递到其符号,可以将其视为相空间上的经典可观察物。通过这种方式,我们获得了等离子运动的有效运动方程。然后,我们使用Einstein-Brilllouin-keller量化找到量化的能级和等离子体光谱。我们的结果提供了一个理论基础,以描述量子等离子间中的不同设置,例如纳米颗粒,量子点和波导。
Recent progress in experimental techniques has made the quantum regime in plasmonics accessible. Since plasmons correspond to collective electron excitations, the electron-electron interaction plays an essential role in their theoretical description. Within the Random Phase Approximation, this interaction is incorporated through a system of equations of motion, which has to be solved self-consistently. For homogeneous media, an analytical solution can be found using the Fourier transform, giving rise to Lindhard theory. When the medium is spatially inhomogeneous, this is no longer possible and one often uses numerical approaches, which are however limited to smaller systems. In this paper, we present a novel semi-analytical approach for bulk plasmons in inhomogeneous media based on the semiclassical (or WKB) approximation, which is applicable when the charge density varies smoothly. By solving the equations of motion self-consistently, we obtain the expressions of Lindhard theory with a spatially varying Fermi wavevector. The derivation involves passing from the operators to their symbols, which can be thought of as classical observables on phase space. In this way we obtain effective (Hamiltonian) equations of motion for plasmons. We then find the quantized energy levels and the plasmon spectrum using Einstein-Brilllouin-Keller quantization. Our results provide a theoretical basis to describe different setups in quantum plasmonics, such as nanoparticles, quantum dots and waveguides.