论文标题
使用卤化物混合的钙钛矿光电探测器的宽带可调光谱响应
Broadband-tunable spectral response of perovskite-on-paper photodetectors using halide mixing
论文作者
论文摘要
纸张为电子产品提供了低成本且可广泛的基板。它具有硅的替代特性,因为它显示出低密度和高柔韧性以及生物降解性。解决方案处理的材料(例如混合钙壶)也具有光和柔性特征,以及具有不同光学特性的材料组成的巨大可调性。在这项研究中,我们将纸基板与卤化物混合的钙钛矿相结合,以创建低成本和易于制作的perovskite-paper-paper光电探测器和宽带可调的光谱响应。从卤化物混合的钙钛矿的带隙可调节性中,我们创建的光电探测器具有截止光谱的发作,从NIR到绿色,通过增加Mapb(i $ _ {1-x} $ br $ _x $)上的溴化物含量来增加溴化物的含量。这些设备显示出快速有效的响应。对于纯I和BR钙钛矿组成,观察到最佳性能,在Mapbbr $ _3 $设备上,最大响应性为376 mA/w。这项研究提供了一个示例,说明了解决方案处理材料与纸基材料的组合提供的各种可能性,以开发低成本,可生物降解和易于制作的设备。
Paper offers a low-cost and widely available substrate for electronics. It posses alternative characteristics to silicon, as it shows low density and high-flexibility, together with biodegradability. Solution processable materials, such as hybrid perovskites, also present light and flexible features, together with a huge tunability of the material composition with varying optical properties. In this study, we combine paper substrates with halide-mixed perovskites for the creation of low-cost and easy-to-fabricate perovskite-on-paper photodetectors with a broadband-tunable spectral response. From the bandgap tunability of halide-mixed perovskites we create photodetectors with a cut-off spectral onset that ranges from the NIR to the green, by increasing the bromide content on MAPb(I$_{1-x}$Br$_x$)$_3$ perovskite alloys. The devices show a fast and efficient response. The best performances are observed for the pure I and Br perovskite compositions, with a maximum responsivity of 376 mA/W on the MAPbBr$_3$ device. This study provides an example of the wide range of possibilities that the combination of solution processable materials with paper substrates offer for the development of low-cost, biodegradable and easy-to-fabricate devices.