论文标题

通过单轴应力调整大量硝酸锂中的域壁电导率

Tuning the domain wall conductivity in bulk lithium niobate by uniaxial stress

论文作者

Singh, Ekta, Beccard, Henrik, Amber, Zeeshan H., Ratzenberger, Julius, Hicks, Clifford W., Rüsing, Michael, Eng, Lukas M.

论文摘要

由于其独特的拓扑,光学和电子特性,在绝缘铁电隔离的导电域壁(CDW)最近引起了广泛的关注,并提供了潜在的应用,例如在存储器设备或重新修订的电路中。域壁(DWS)的电子性能可以通过施用应变来调节,因此可以控制DWS处的电荷载体密度。在这项工作中,我们研究了单轴应力对散装单晶硅锂(Linbo $ _3 $)中DW电导率的影响。使用导电原子力显微镜(CAFM),我们观察到DWS的电导率中存在较大的不对称性,在该电导率下,只有负屏蔽的壁(所谓的头对头DWS)变得越来越多地导电,同时进行了积极的筛选,尾巴到尾dws的电导率下降。 DW电导率的这种不对称性与我们基于压电效应的理论模型一致。此外,我们观察到DW中的电流增加到一个数量级,对于100 MPa的较小压缩应力。在2个月内,DWS的这种反应仍然完好无损,为将来的应用打开了一条途径。

Conductive domain walls (CDWs) in insulating ferroelectrics have recently attracted considerable attention due to their unique topological, optical, and electronic properties, and offer potential applications such as in memory devices or re-writable circuitry. The electronic properties of domain walls (DWs) can be tuned by the application of strain, hence controlling the charge carrier density at DWs. In this work, we study the influence of uniaxial stress on the conductivity of DWs in the bulk single crystal lithium niobate (LiNbO$_3$). Using conductive atomic force microscopy (cAFM), we observe a large asymmetry in the conductivity of DWs, where only negatively screened walls, so called head-to-head DWs, are becoming increasingly conductive, while positively screened, tail-to-tails DWs, show a decrease in conductivity. This asymmetry of DW conductivity agrees with our theoretical model based on the piezoelectric effect. In addition, we observed that the current in the DW increases up to an order of magnitude for smaller compressive stresses of 100 MPa. This response of DWs remained intact for multiple stress cycles over 2 months, opening a path for future applications.

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