论文标题

铁磁合金中全光超快开关过程的现实微磁性描述

Realistic micromagnetic description of all-optical ultrafast switching processes in ferrimagnetic alloys

论文作者

Raposo, V., García-Sánchez, F., Atxitia, U., Martínez, E.

论文摘要

由单个超短激光脉冲驱动的螺旋性无关和螺旋依赖性的全光开关过程已在铁磁合金中被实验证明,为GDFECO。尽管先前已通过原子模拟再现了转换,但是缺乏用于铁磁体的鲁棒微型框架将预测限制为小纳米系统的预测,而实验通常是用激光器和小米的样品进行的。在这里,我们开发了一个基于扩展的Landau-Lifshitz-Bloch方程的微磁模型,该模型首先通过直接重现小样品和均匀激光加热的原子效果来验证。之后,该模型用于研究在逼真的条件下铁磁合金中的超快单镜头全光开关。我们发现,在线性极化激光脉冲下,无螺旋性无关开关是一种纯热现象,其中倒置区域的大小与样品中的最大电子温度直接相关。另一方面,对具有不同组成的铁磁合金中的圆形极化脉冲下的螺旋性依赖性过程的分析表明,磁圆二色​​性和反向法拉第效应的结果之间的质量差异。基于这些预测,我们提出了实验,以解决基于这些螺旋性依赖所有光学过程的物理现象的争议。

Both helicity-independent and helicity-dependent all-optical switching processes driven by single ultrashort laser pulse have been experimentally demonstrated in ferrimagnetic alloys as GdFeCo. Although the switching has been previously reproduced by atomistic simulations, the lack of a robust micromagnetic framework for ferrimagnets limits the predictions to small nano-systems, whereas the experiments are usually performed with lasers and samples of tens of micrometers. Here we develop a micromagnetic model based on the extended Landau-Lifshitz-Bloch equation, which is firstly validated by directly reproducing atomistic results for small samples and uniform laser heating. After that, the model is used to study ultrafast single shot all-optical switching in ferrimagnetic alloys under realistic conditions. We find that the helicity-independent switching under a linearly polarized laser pulse is a pure thermal phenomenon, in which the size of inverted area directly correlates with the maximum electron temperature in the sample. On the other hand, the analysis of the helicity-dependent processes under circular polarized pulses in ferrimagnetic alloys with different composition indicates qualitative differences between the results predicted by the magnetic circular dichroism and the ones from inverse Faraday effect. Based on these predictions, we propose experiments that would allow to resolve the controversy over the physical phenomenon that underlies these helicity-dependent all optical processes.

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