论文标题
条纹铜层中的光学引起的umklapp偏移电流
Optically-induced Umklapp shift currents in striped cuprates
论文作者
论文摘要
在最近的实验中,在掺杂的条纹超导体中观察到低频二阶光学响应的动机,在这里我们研究了表现出电荷密度波(CDW)顺序参数的系统的非线性电动力学。由于Bragg散射CDW顺序,除了零动量电流外,传入的空间均匀电场还会产生umklapp电流,这些电流在相互cdw晶格的矩矩处调节。特别是,我们在这里预测和显微镜评估了Umklapp Shift电流,Umklapp Shift电流是常规移位电流的有限动量类似物,该电流代表了将均匀的AC电场下调为低频,零动量电流的二阶光学过程。具体而言,我们通过Keldysh技术评估平均场理论中的实时响应函数,并使用PEIERLS替换来计算晶格模型中有限动量的可观察物。我们发现,具有某些晶格对称性的系统(例如反转对称性)可能会导致umklapp一个。我们将框架应用于带有螺旋状条纹的分层材料中的晶格对称性,并表明两种类型的转移电流都可以洞悉物质相互论形阶段的性质。最后,我们讨论了我们的发现与条纹超导体最新实验的关系。
Motivated by recent experiments that observed low-frequency second-order optical responses in doped striped superconductors, here we investigate the nonlinear electrodynamics of systems exhibiting a charge density wave (CDW) order parameter. Due to the Bragg scattering off the CDW order, an incoming spatially homogeneous electric field in addition to zero momentum current generates Umklapp currents that are modulated in space at momenta of the reciprocal CDW lattice. In particular, here we predict and microscopically evaluate the Umklapp shift current, a finite momentum analog of the regular shift current which represents the second-order optical process that downconverts homogeneous AC electric field into low-frequency, zero momentum current. Specifically, we evaluate real-time response functions within mean-field theory via the Keldysh technique and use the Peierls substitution to compute observables at finite momenta in lattice models. We find that systems with certain lattice symmetries (such as inversion symmetry), where the regular shift current is disallowed, may give rise to the Umklapp one. We apply our framework to investigate lattice symmetries in layered materials with helical-like stripes and show that both types of shift currents provide insight into the nature of intertwined phases of matter. Finally, we discuss the relation of our findings to recent experiments in striped superconductors.