论文标题
粘合剂相互作用对植物凝胶中应变僵硬和耗散的影响
Effect of adhesive interaction on strain stiffening and dissipation in granular gels undergoing yielding
论文作者
论文摘要
压力引起的无序固体中的屈服/流体化,其特征是不可逆性和增强耗散,对于广泛的工业和地质过程至关重要。尽管热系统中的这种现象已经进行了广泛的研究,但对于颗粒状固体而言,它们对它们的理解仍然很差。在这里,使用振荡性剪切流变学和原位光学成像,我们研究了粘合剂颗粒的致密颗粒悬浮液中的能量耗散,这些粘合剂颗粒的颗粒状悬浮液产生的压力固体远低于远低于硬球抑制限制的各向同性堵塞点。我们发现有趣的非线性流动机制,包括周期内应变僵硬和可塑性,这在很大程度上取决于应用应变振幅($γ_0$)和粒子体积分数($ ϕ $)。我们证明,在整个参数范围内的这种非线性可以通过称为归一化能量耗散($ e_n $)的无量纲变量有效地捕获。此外,原位光学成像揭示了与局部速度的时空波动相关的不可逆粒子重排,其性质在整个屈服过渡过程中都有明显的变化。通过使用粒子沉降实验直接测量关键的干扰堆积分数,我们提出了一个详细的相图,该相图揭示了跨颗粒相互作用在控制系统流量范围内的$γ_0$和$ $ ϕ $值的作用。
Stress induced yielding/fluidization in disordered solids, characterized by irreversibility and enhanced dissipation, is important for a wide range of industrial and geological processes. Although, such phenomena in thermal systems have been extensively studied, they remain poorly understood for granular solids. Here, using oscillatory shear rheology and in-situ optical imaging, we study energy dissipation in a dense granular suspension of adhesive particles that forms yield stress solids far below the isotropic jamming point obtained in the limit of hard-sphere repulsion. We find interesting non-linear flow regimes including intra-cycle strain stiffening and plasticity that strongly depend on the applied strain amplitude ($γ_0$) and particle volume fraction ($ϕ$). We demonstrate that such nonlinearity over the entire parameter range can be effectively captured by a dimensionless variable termed as the normalized energy dissipation ($E_N$). Furthermore, in-situ optical imaging reveals irreversible particle rearrangements correlating with the spatiotemporal fluctuations in local velocity, the nature of which strikingly varies across the yielding transition. By directly measuring the critical jamming packing fractions using particle settling experiments, we propose a detailed phase diagram that unravels the role of inter-particle interactions in controlling the flow properties of the system for a wide range of $γ_0$ and $ϕ$ values.