论文标题

kagome超导体CSV $ _ {3} $ sb $ _ {5} $的薄片中的大量子振荡频率的出现

Emergence of large quantum oscillation frequencies in thin flakes of the kagome superconductor CsV$_{3}$Sb$_{5}$

论文作者

Zhang, W., Wang, Lingfei, Tsang, Chun Wai, Liu, Xinyou, Xie, Jianyu, Yu, Wing Chi, Lai, Kwing To, Goh, Swee K.

论文摘要

Kagome金属AV $ _3 $ SB $ _5 $〜(A = K,RB,CS)最近被发现的平台具有不寻常的电荷密度波(CDW)订单和超导性。 kagome晶格的电子带结构可以容纳平坦带和类似狄拉克的带,从而提供了稳定各种量子状态的可能性。在这里,我们通过Shubnikov-de haas量子振荡探测CSV $ _3 $ sb $ _5 $的频带结构。尽管我们的频谱与已发布的数据广泛一致,但我们明确地揭示了新频率的存在,其频率从$ \ sim $ 2085〜T到$ \ sim $ \ sim $ 2717〜当磁场沿着$ c $轴时。这些准二维频率对应于$ \ sim $ 52 \%至67 \%\%的CDW延伸的Brillouin区域体积。对于这些频率,LIFSHITZ-KOSEVICH分析进一步发现了令人惊讶的小回旋有效质量,$ \ sim $ 0.1〜 $ m_e $的顺序。因此,在CSV $ _3 $ _3 $ sb $ _5 $的薄片中存在大量高速载体。与我们的频带结构计算相比,我们认为轨道结构的轨道选择性修饰是活跃的。我们的结果提供了必不可少的信息,以了解CSV $ _3 $ SB $ _5 $的费米学,铺平了一种理解轨道选择机制如何成为调整其电子属性的有效手段的方法。

Kagome metals AV$_3$Sb$_5$~(A = K, Rb, Cs) are recently discovered platforms featuring an unusual charge-density-wave (CDW) order and superconductivity. The electronic band structure of a kagome lattice can host both flat bands as well as Dirac-like bands, offering the possibility to stabilize various quantum states. Here, we probe the band structure of CsV$_3$Sb$_5$ via Shubnikov-de Haas quantum oscillations on both bulk single crystals and thin flakes. Although our frequency spectra are broadly consistent with the published data, we unambiguously reveal the existence of new frequencies with large frequencies ranging from $\sim$2085~T to $\sim$2717~T in thin flakes when the magnetic field is along the $c$-axis. These quasi-two-dimensional frequencies correspond to $\sim$52\% to 67\% of the CDW-distorted Brillouin zone volume. The Lifshitz-Kosevich analysis further uncovers surprisingly small cyclotron effective masses, of the order of $\sim$0.1~$m_e$, for these frequencies. Consequently, a large number of high-velocity carriers exists in the thin flake of CsV$_3$Sb$_5$. Comparing with our band structure calculations, we argue that an orbital-selective modification of the band structure is active. Our results provide indispensable information for understanding the fermiology of CsV$_3$Sb$_5$, paving a way for understanding how an orbital-selective mechanism can become an effective means to tune its electronic properties.

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