论文标题

收费订单景观和竞争与Kagome金属的超导性

Charge order landscape and competition with superconductivity in kagome metals

论文作者

Kang, Mingu, Fang, Shiang, Yoo, Jonggyu, Ortiz, Brenden R., Oey, Yuzki, Choi, Jonghyeok, Ryu, Sae Hee, Kim, Jimin, Jozwiak, Chris, Bostwick, Aaron, Rotenberg, Eli, Kaxiras, Efthimios, Checkelsky, Joseph G., Wilson, Stephen D., Park, Jae-Hoon, Comin, Riccardo

论文摘要

在Kagome金属AV3SB5(A = K,RB,CS)中,三维电荷顺序(3D-CO)是主要的不稳定性,它为其他集体订单奠定了阶段,包括单向条纹顺序,轨道通量,轨道磁通序,电子性nematoric nematicitient and ExprySconcantivity。在这里,我们使用高分辨率角度分辨的光发射光谱来确定AV3SB5中三维电荷顺序(3D-CO)的显微镜结构及其与超导性的相互作用。我们的方法是基于确定由3D-CO诱导的kagome带的异常分裂,该kagome带提供了一种敏感的方法来完善相邻的kagome平面中的空间电荷模式。我们发现3D-CO结构对组成和掺杂的明显依赖性。观察到的CSV3SB5与其他化合物之间的差异可能是CSV3(SB,SN)5中的双层超导性的基础,以及KV3SB5和RBV3SB5中TC的抑制。我们的结果为AV3SB5的丰富相图提供了新的见解。

In kagome metals AV3Sb5 (A = K, Rb, Cs), three-dimensional charge order (3D-CO) is the primary instability that sets the stage for other collective orders to emerge, including unidirectional stripe order, orbital flux order, electronic nematicity, and superconductivity. Here, we use high-resolution angle-resolved photoemission spectroscopy to determine the microscopic structure of three-dimensional charge order (3D-CO) in AV3Sb5 and its interplay with superconductivity. Our approach is based on identifying an unusual splitting of kagome bands induced by 3D-CO, which provides a sensitive way to refine the spatial charge patterns in neighboring kagome planes. We found a marked dependence of the 3D-CO structure on composition and doping. The observed difference between CsV3Sb5 and the other compounds potentially underpins the double-dome superconductivity in CsV3(Sb,Sn)5 and the suppression of Tc in KV3Sb5 and RbV3Sb5. Our results provide fresh insights into the rich phase diagram of AV3Sb5.

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