论文标题
旋转激发光谱中的依赖电压依赖性对称性破坏效果 - $ \ frac {1} {2} $ parmagnetic分子连接从平衡中驱动的
Voltage Dependent Symmetry Breaking Effects in the Spin Excitation Spectrum of Spin-$\frac{1}{2}$ Paramagnetic Molecular Junctions Driven Out of Equilibrium
论文作者
论文摘要
在目前的工作中,我们考虑了一个旋转1/2的顺磁性二聚体,该二聚体嵌入了磁性隧道连接中,在存在外部磁性偏置的情况下,通过施加的电压和施加的温度梯度通过施加的电压和施加的温度梯度从平衡中驱动,可以打开/关闭。在这里,我们通过分析两个自旋1/2系统的自旋激发光谱得出了自旋激发光谱,并表明需要外部磁场来提高三胞胎状态的退化,无论两个旋转单元是否在相同的方向上还是在相反的交错方向上经历磁场。我们表明,在没有磁场的情况下,施加的偏置电压将磁性从磁导线转移到分子中嵌入的旋转单元中,因此在没有外部磁力的情况下破坏了对称性并提升了三重态。从理论上的演示中,我们提出了两种磁性驱动方案,以提高自旋激发光谱中的自旋退化,我们将其命名为PMD(平行磁性驱动)和AMD(反平行磁性驱动)。我们认为,需要进行对称性破坏,以将二聚体的自旋构型投射到量子传输测量中,因此提出了不同的方案,以检测自旋三胞胎状态和旋转单元素状态,并使用非降级的非对称型号的旋转电导率测量结果与我们的结果相比,将其与文献相比。
In the present work, we consider a spin 1/2 paramagnetic dimer embedded in a magnetic tunnel junction driven out of equilibrium by means of an applied voltage and an applied temperature gradient, in the presence of an external magnetic bias, which can be turn on/off. Here, we derive the spin excitation spectrum for a two spin 1/2 system analytically and show that an external magnetic field is required to lift the degeneracy in the triplet state, whether both spin units experience the magnetic field in the same direction or in opposite staggered directions. We show that an applied bias voltage in the absence of a magnetic field, transfers the magnetization from the magnetic leads into the spin units embedded in the molecule, hence breaking a symmetry and lifting the triplet degeneracy in the absence of external magnetization. From this theoretical demonstration, we then propose two schemes of magnetic driving to lift spin degeneracy in the spin excitation spectrum, which we named PMD (Parallel Magnetic Driving) and AMD (Anti-Parallel Magnetic Driving). We argue that a symmetry breaking is then required to project the spin configuration of a dimer into quantum transport measurements, and hence propose different schemes to detect the spin triplet state and the spin singlet state using differential conductivity measurements in the non-degenerate non-symmetric configuration of the spin dimer, and compare our results with the ones reported in the literature.