论文标题

将单层AG作为大差距2D半导体,其动量解决了激发态

Confined monolayer Ag as a large gap 2D semiconductor and its momentum resolved excited states

论文作者

Lee, Woojoo, Wang, Yuanxi, Qin, Wei, Kim, Hyunsue, Liu, Mengke, Nunley, T. Nathan, Fang, Bin, Maniyara, Rinu, Dong, Chengye, Robinson, Joshua A., Crespi, Vincent, Li, Xiaoqin, MacDonald, Allan H., Shih, Chih-Kang

论文摘要

2D材料具有吸引人的量子现象,与它们的批量不同。最近,由元素原子组成的外延合成的晶圆尺度2D金属不仅吸引了其潜在应用,而且吸引了诸如超导性等外来量子效应。通过使用时间分辨和角度分辨光发射光谱(ARPES)绘制动量分辨的电子状态,我们揭示了限制在Biyerer Graphene和SIC之间的单层Ag是一个较大的差距(> 1 eV)2D半导体,与GW纠正的密度密度功能理论一致。测得的价带分散匹配DFT-GW准粒子带。但是,传导带分散剂显示出异常的有效质量为2.4 m0。讨论了明显质量中这种大型增强的可能机制。

2D materials have intriguing quantum phenomena that are distinctively different from their bulk counterparts. Recently, epitaxially synthesized wafer-scale 2D metals, composed of elemental atoms, are attracting attention not only for their potential applications but also for exotic quantum effects such as superconductivity. By mapping momentum-resolved electronic states using time-resolved and angle-resolved photoemission spectroscopy (ARPES), we reveal that monolayer Ag confined between bilayer graphene and SiC is a large gap (> 1 eV) 2D semiconductor, consistent with GW-corrected density functional theory. The measured valence band dispersion matches the DFT-GW quasiparticle band. However, the conduction band dispersion shows an anomalously large effective mass of 2.4 m0. Possible mechanisms for this large enhancement in the apparent mass are discussed.

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