论文标题

通过NMR绘制共掺杂的Lafeaso单晶的自旋波动

Mapping out the spin fluctuations in Co-doped LaFeAsO single crystals by NMR

论文作者

Lepucki, Piotr, Havemann, Raphael, Dioguardi, Adam P., Scaravaggi, Francesco, Wolter-Giraud, Anja U. B., Kappenberger, Rhea, Aswartham, Sai, Wurmehl, Sabine, Büchner, Bernd, Grafe, Hans-Joachim

论文摘要

我们通过使用核磁共振(NMR)来确定Lafe $ _ {1-X} $ CO $ _X $ ASO单晶的相位图。最多达到$ x = 0.03 $的名义掺杂,它遵循F掺杂多晶的相图。高于$ x = 0.03 $,F掺杂样品成为超导,而对于共同掺杂结构和磁过渡,可以观察到$ x = 0.042 $,并且超导性仅用于较高的兴奋剂水平,并且过渡温度降低。对于最大$ x = 0.056 $的兴奋剂,我们找到了短距离磁性顺序的证据。通过弛豫率测量,我们绘制出揭示了nematicity和磁性相互作用的磁波动。在上面的订购之上,Lafe $ _ {1-x} $ co $ _x $ aso中的自旋波动与BA(Fe $ _ {1-x} $ _x $ _x $)$ _ 2 $ as $ _2 $相同,这表明Lafeaso中的nematicity在Lafeaso中是一种结果,这是一个造成的旋转旋转wave。

We determine the phase diagram of LaFe$_{1-x}$Co$_x$AsO single crystals by using nuclear magnetic resonance (NMR). Up to a nominal doping of $x=0.03$, it follows the phase diagram for F-doped polycrystals. Above $x=0.03$, the F-doped samples become superconducting, whereas for Co-doping the structural and magnetic transitions can be observed up to $x=0.042$, and superconductivity occurs only for higher doping levels and with reduced transition temperatures. For dopings up to $x=0.056$, we find evidence for short-range magnetic order. By means of relaxation-rate measurements, we map out the magnetic fluctuations that reveal the interplay of nematicity and magnetism. Above the nematic ordering, the spin fluctuations in LaFe$_{1-x}$Co$_x$AsO are identical to those in Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$, suggesting that nematicity in LaFeAsO is a result of the fluctuating spin density wave as well.

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