论文标题
原子蒸气中的圆二色性:磁引起的过渡,导致了两种不同的行为
Circular dichroism in atomic vapors: magnetically induced transitions responsible for two distinct behaviors
论文作者
论文摘要
满足条件$ f_e-f_g = \ pm2 $的碱金属的原子过渡,在零磁场中的概率为无概率,而当应用外部场时可能会增加巨大增加。这种过渡通常被称为磁引起的(MI)过渡,因为它们在宽的外部磁场范围内的概率很高,在某些情况下,这些概率甚至高于通常的原子过渡。以前,建立了以下规则:使用$ΔF= \ pm2 $的MI过渡的强度分别使用$σ^\ pm $辐射时最大。在相同的基态内,$σ^+$和$σ^ - $辐射的强度差异可能很重要,导致磁性诱导的圆二色性(MCD),称为1型。在这里,我们表明,即使是最强的MI过渡中的$,即以$σ^ + $和$σ^ - $的不同地面状态$ $,$ΔF= + 2 $的MI过渡的概率总是更大的,这会导致另一种类型的MCD。我们的实验是使用CS填充的纳米赛执行的,该纳米孔在D $ _2 $行周围调节激光器。其他碱金属的预期也有类似的结果。理论计算与实验测量非常吻合。
Atomic transitions of alkali metals for which the condition $F_e-F_g = \pm2$ is satisfied have null probability in a zero magnetic field, while a giant increase can occur when an external field is applied. Such transitions, often referred to as magnetically-induced (MI) transitions, have received interest because their high probabilities in wide ranges of external magnetic fields which, in some cases, are even higher than that of usual atomic transitions. Previously, the following rule was established: the intensities of MI transitions with $ΔF=\pm2$ are maximum when using respectively $σ^\pm$ radiation. Within the same ground state, the difference in intensity for $σ^+$ and $σ^-$ radiations can be significant, leading to magnetically induced circular dichroism (MCD), referred to as type-1. Here, we show that even among the strongest MI transitions, $i.e$ originating from different ground states for $σ^+$ and $σ^-$, the probability of MI transition with $ΔF = + 2$ is always greater, which leads to another type of MCD. Our experiments are performed with a Cs-filled nanocell, where the laser is tuned around the D$_2$ line; similar results are expected with other alkali metals. Theoretical calculations are in excellent agreement with the experimental measurements.