论文标题
光锥中单层WSE2中激子精细结构的伪旋转纹理的光学测量
Optical Measurement of Pseudo-Spin Texture of the Exciton Fine-Structure in Monolayer WSe2 within the Light Cone
论文作者
论文摘要
几个理论上的预测声称,TMDC的中性激子分裂为横向和纵向激子分支,纵向上的一个是上部分支,在光锥内的MEV范围内表现出非凡的强分散体。从历史上看,这与半导体量子孔连接到了强场光学偶极子偶联或强烈的电子远程交换相互作用,描述了同一硬币的两个侧面。最近,利用傅立叶空间光谱法的实验表明,确实可以测量激子(激子 - 帕利顿)分散剂的高质量六边形-BN包裹的WSE2单层样品,并可以确认能量量表。在这里,研究了激子精细结构的伪旋转和山谷极化,这是质量中心和激发激光失调的函数的函数。对于准召唤激发,观察到具有明显动量依赖性螺旋的强烈分散体。通过将激发能量逐步增加对电子带隙的逐步增加,由于不一致的激子和血浆发射的贡献,分散和螺旋性会系统地降低。使用巨质质量的质量下降,可以通过Maialle-Silva-SHAM机制在现象学上使用激子拆分作为有效磁场的来源来建模。
Several theoretical predictions have claimed that the neutral exciton of TMDCs splits into a transversal and longitudinal exciton branch, with the longitudinal one, which is the upper branch, exhibiting an extraordinary strong dispersion in the meV range within the light cone. Historically, this was linked for semiconductor quantum wells to strong far-field optical dipole coupling, or strong electronic long-range exchange interactions, describing two sides of the same coin. Recently, experiments utilizing Fourier-space spectroscopy have shown that the exciton (exciton-polariton) dispersion can indeed be measured for high-quality hexagonal-BN-encapsulated WSe2 monolayer samples and can confirm the energy scale. Here, the exciton fine-structure's pseudo-spin and the valley polarization are investigated as a function of the centre-of-mass-momentum and excitation-laser detuning. For quasi-resonant excitation, a strong dispersion featuring a pronounced momentum-dependent helicity is observed. By increasing the excitation energy step-wise towards and then above the electronic band gap, the dispersion and the helicity systematically decrease due to contributions of incoherent excitons and emission from plasma. The decline of the helicity with centre-of-mass momentum can be phenomenologically modelled by the Maialle-Silva-Sham mechanism using the exciton splitting as the source of an effective magnetic field.