论文标题

CRBR $ _3 $ _3 $的磁性van der waals异质结构中的旋转热量

Spin caloritronics in a CrBr$_3$-based magnetic van der Waals heterostructure

论文作者

Liu, Tian, Peiro, Julian, de Wal, Dennis K., Leutenantsmeyer, Johannes C., Guimarães, Marcos H. D., van Wees, Bart J., work, These authors contributed equally to this

论文摘要

最近报道的磁性顺序用于绝缘二维(2D)材料,例如三碘化物(CRI $ _3 $)和TRIBRomIDE铬(CRBR $ _3 $),为基于2D系统的磁铁电子设备的制造开辟了新的可能性。不可避免地,2D磁铁中的磁化和自旋动力学与焦耳加热密切相关。因此,了解自旋,电荷和热量之间的耦合,即自旋热量效应至关重要。然而,由于空气中的不稳定,2D铁磁体中的自旋热量量很大。在这里,我们开发了一种制造方法,该方法通过HBN封装将自旋活动接触与2D磁铁整合在一起,从而使我们能够探索这些材料中的旋转热量效应。研究了磁场和加热电流的不同条件,研究了CRBR $ _3 $/PT系统的热自旋信号的角度依赖性。我们强调了pt中异常的nernst效果揭示的Crbr $ _3 $在PT上存在显着的磁接近效应,并提出了CRBR $ _3 $的自旋Seebeck效应的贡献。这些结果使用空气敏感的2D磁绝缘子为将来的宏伟设备铺平了道路。

The recently reported magnetic ordering in insulating two-dimensional (2D) materials, such as chromium triiodide (CrI$_3$) and chromium tribromide (CrBr$_3$), opens new possibilities for the fabrication of magneto-electronic devices based on 2D systems. Inevitably, the magnetization and spin dynamics in 2D magnets are strongly linked to Joule heating. Therefore, understanding the coupling between spin, charge and heat, i.e. spin caloritronic effects, is crucial. However, spin caloritronics in 2D ferromagnets remains mostly unexplored, due to their instability in air. Here we develop a fabrication method that integrates spin-active contacts with 2D magnets through hBN encapsulation, allowing us to explore the spin caloritronic effects in these materials. The angular dependence of the thermal spin signal of the CrBr$_3$/Pt system is studied, for different conditions of magnetic field and heating current. We highlight the presence of a significant magnetic proximity effect from CrBr$_3$ on Pt revealed by an anomalous Nernst effect in Pt, and suggest the contribution of the spin Seebeck effect from CrBr$_3$. These results pave the way for future magnonic devices using air-sensitive 2D magnetic insulators.

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