论文标题

YMNO $ _3 $中不正确的铁电域的本地控制

Local control of improper ferroelectric domains in YMnO$_3$

论文作者

Kuerten, Lukas, Krohns, Stephan, Schoenherr, Peggy, Holeczek, Katharina, Pomjakushina, Ekaterina, Lottermoser, Thomas, Trassin, Morgan, Meier, Dennis, Fiebig, Manfred

论文摘要

铁电的不当用两个阶参数描述:主要的参数,驱动向远程扭曲,磁或其他非电动阶的过渡,而电偏振是由主要阶参数引起的,作为次级参数作为次要的互补效应。使用低温扫描探针显微镜,我们表明YMNO $ _3 $中的铁电域不当,可以通过电场极点局部切换。但是,随后的温度变化恢复了由原发晶格失真确定的生长域结构。由于在低温下缺乏移动筛查费用,在新书面的域墙壁上发生了无偿的界定电荷来解释反向交换。因此,在许多方面,不当铁电体的极化受到与适当对应物相同的静电的影响,但与主要阶参数引起的其他功能相辅相成。因此,定制主要阶参数,极化和静电之间的复杂相互作用可能会导致针对不当铁电的新功能。

Improper ferroelectrics are described by two order parameters: a primary one, driving a transition to long-range distortive, magnetic or otherwise non-electric order, and the electric polarization, which is induced by the primary order parameter as a secondary, complementary effect. Using low-temperature scanning probe microscopy, we show that improper ferroelectric domains in YMnO$_3$ can be locally switched by electric field poling. However, subsequent temperature changes restore the as-grown domain structure as determined by the primary lattice distortion. The backswitching is explained by uncompensated bound charges occuring at the newly written domain walls due to the lack of mobile screening charges at low temperature. Thus, the polarization of improper ferroelectrics is in many ways subject to the same electrostatics as in their proper counterparts, yet complemented by additional functionalities arising from the primary order parameter. Tailoring the complex interplay between primary order parameter, polarization, and electrostatics is therefore likely to result in novel functionalities specific to improper ferroelectrics.

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