论文标题
NBN超导体中第三次谐波产生中的HIGGS模式共振:多播电子偶联,杂质散射和极化角度依赖性
Higgs-mode resonance in third harmonic generation in NbN superconductors: multiband electron-phonon coupling, impurity scattering, and polarization-angle dependence
论文作者
论文摘要
从理论上讲,我们研究了第三次谐波产生(THG)的共振,这些共振在多摩德无序超导体NBN中的频率是超导间隙的一半。中心问题是对THG共振的主要贡献是来自Higgs模式(超导顺序参数的集体振幅模式)还是Quasiparticle激发。为了解决这个问题,我们分析了一个现实的三波段模型,该模型具有有效的贴纸上和频带介导的相互作用,从第一原理估算了与非磁性杂质散射。使用估计的配对相互作用与多型杂质散射率的差异从干净到肮脏的机制变化,我们通过BCS和自以为是的Born近似值以通道分辨的方式计算NBN的THG易感性。在接近实验情况的肮脏状态中,主要的贡献是由希格斯模式的顺磁通道给出的,几乎没有极化角度依赖性,而第二个主要贡献来自准粒子的顺磁通道,通常显示出显着的极化依赖性。结果与最近对无极化角度依赖性的实验观察一致,这证明了HIGGS模式主要有助于NBN超导体的THG共振。
We theoretically investigate the resonance of third harmonic generation (THG) that has been observed at frequency being half of the superconducting gap in a multiband disordered superconductor NbN. The central question is whether the dominant contribution to the THG resonance comes from the Higgs mode (the collective amplitude mode of the superconducting order parameter) or quasiparticle excitations. To resolve this issue, we analyze a realistic three-band model with effective intraband and interband phonon-mediated interactions estimated from first-principles together with nonmagnetic impurity scatterings. Using the estimated pairing interactions with multiband impurity scattering rates being varied from clean to dirty regimes, we calculate the THG susceptibility for NbN in a channel-resolved manner by means of the BCS and self-consistent Born approximations. In the dirty regime, which is close to the experimental situation, the leading contribution is given by the paramagnetic channel of the Higgs mode having almost no polarization-angle dependence, while the second leading contribution comes from the paramagnetic channel of quasiparticles generally showing significant polarization-angle dependence. The result is consistent with the recent experimental observation of no polarization-angle dependence of THG, giving firm evidence that the Higgs mode dominantly contributes to the THG resonance in NbN superconductors.