论文标题

基于钻石的宽场热成像的最佳体系结构

Optimal architecture for diamond-based wide-field thermal imaging

论文作者

Tanos, R., Akhtar, W., Monneret, S., de Oliveira, F. Favaro, Seniutinas, G., Munsch, M., Maletinsky, P., Gratiet, L. le, Sagnes, I., Dréau, A., Gergely, C., Jacques, V., Baffou, G., Robert-Philip, I.

论文摘要

钻石中的氮气视口中心具有很大取决于温度的电子自旋共振,这使它们具有有效的温度传感器,其灵敏度降至几个Mk/$ \ sqrt {\ rm Hz} $。然而,宿主钻石的高热电导率可能会强烈潮湿任何温度变化,从而在探测局部温度分布时会导致侵入性测量。鉴于确定基于钻石的宽场热成像的可能和最佳构型,我们在这里在实验和数字上研究了钻石的存在对显微镜温度分布的影响。研究了三种几何构型:散装钻石底物,薄的钻石层在石英和钻石纳米颗粒上分散在石英上。我们表明,在这种意义上,将大量钻石底物用于热成像是高度侵入性的,因为它可以防止任何大幅度的温度升高。相反,薄钻石层部分解决了此问题,可以为微观热成像提供可能的替代方法。钻石纳米颗粒在整个样品中的分散是最相关的方法,因为它们不影响温度分布,尽管与散装钻石相比,纳米座中心的NV中心产生的温度敏感性较低。

Nitrogen-Vacancy centers in diamond possess an electronic spin resonance that strongly depends on temperature, which makes them efficient temperature sensor with a sensitivity down to a few mK/$\sqrt{\rm Hz}$. However, the high thermal conductivity of the host diamond may strongly damp any temperature variations, leading to invasive measurements when probing local temperature distributions. In view of determining possible and optimal configurations for diamond-based wide-field thermal imaging, we here investigate, both experimentally and numerically, the effect of the presence of diamond on microscale temperature distributions. Three geometrical configurations are studied: a bulk diamond substrate, a thin diamond layer bonded on quartz and diamond nanoparticles dispersed on quartz. We show that the use of bulk diamond substrates for thermal imaging is highly invasive, in the sense that it prevents any substantial temperature increase. Conversely, thin diamond layers partly solve this issue and could provide a possible alternative for microscale thermal imaging. Dispersions of diamond nanoparticles throughout the sample appear as the most relevant approach as they do not affect the temperature distribution, although NV centers in nanodiamonds yield lower temperature sensitivities compared to bulk diamond.

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