论文标题
在渠道限制的列流中对拓扑状态的微流体控制
Microfluidic control over topological states in channel-confined nematic flows
论文作者
论文摘要
与各向同性液体相比,列明液晶的定向顺序使其流变特性更加参与,因此需要对流程参数进行精心控制以控制定向模式。在具有垂直表面比对的微流体通道中,在低流速下从低流速下的垂直结构到高流速的流量对齐结构的近亲nematics不连续过渡。在这里,我们展示了如何使用驾驶压力的精确调整来稳定和操纵先前未经研究的拓扑保护的手性手性中间状态,该状态在同型旋转之前出现到流动对准的过渡。我们表征了过渡的基础机制,并构建了一个现象学模型,以描述观察到的手性流动状态的临界行为和相图,并通过引入手性掺杂剂来评估强制对称性破坏的效果。最后,我们通过通道几何形状,激光镊子的应用以及仔细控制流量来诱导需求过渡。
Compared to isotropic liquids, orientational order of nematic liquid crystals makes their rheological properties more involved, and thus requires fine control of the flow parameters to govern the orientational patterns. In microfluidic channels with perpendicular surface alignment, nematics discontinuously transition from perpendicular structure at low flow rates to flow-aligned structure at high flow rates. Here we show how precise tuning of the driving pressure can be used to stabilize and manipulate a previously unresearched topologically protected chiral intermediate state which arises before the homeotropic to flow-aligned transition. We characterize the mechanisms underlying the transition and construct a phenomenological model to describe the critical behaviour and the phase diagram of the observed chiral flow state, and evaluate the effect of a forced symmetry breaking by introduction of a chiral dopant. Finally, we induce transitions on demand through channel geometry, application of laser tweezers, and careful control of the flow rate.